I just remembered, I once had a similar thing that sounded like excessive valve clearence. In the end, it turned out to be a broken valve spring! This way the claerence was ok, but the spring tension too weak so the valve would bounce. As it was the inner springand it was split lengthwise to the wire, it wasn't even visible before disassembly. The result wasquite a chatter and I'd recon this might be worse in certain rpms.
Or maybe it's really just worn valve springs. Have you measured the length and tension yet?